Copyright 1999 by Andrew Bach

Assistant Professor, Western Washington University

Notes on Paleoenvironmental Reconstructions with Soils
DATING TECHNIQUES: Geog. 432 Soils Bach
1. Calendar
2. Review Terminology
a. stratigraphic vs. SED
b. Numerical/Correlated/Calibrated/Relative

3. Dendrochrology
4. Varves
5. Radiocarbon Dating
6. K-Ar Dating
7. Uranium-Series
8.Tephrachronology
9. Paleomagnetism
10. Obsidian (and tephra) Hydration Dating
11. Thermoluminescence (TL)
12. Amino Acid Racemization (AAR)
13. Soils as a Dating Tool
Birkeland - Soil Stratigraphy
Harden- Soil Index
Ca-carbonate: Model, C-14, U-trend, U-series

14. Varnish
15. In Situ Cosmogenic Isotopes

2a. stratigraphic vs. SED

* Explain basic distinction

* Earth & Archaeological Sciences based on stratigraphic.
Almost a paradigm in the methodology.
Affects sampling, interpretation, funding, future work.

b. Numerical/Correlated/Calibrated/Relative

3. Dendrochrology
Basic idea: in seasonal climates of mid- and high-latitudes yearly growth rings are prominent. Each ring is formed by larger cells and softer wood formed in spring and smaller/denser cells in summer and autumn.

5. Radiocarbon Dating
Carbon-14 atoms form in the earth atmosphere from cosmic ray bombardment, mostly protons from elsewhere in the galaxy.

- radiometric OK. Relates to spontaneous radioactibe decay by loss of alpha (helium atom, 2 protons & 2 neutrons) or Beta (electrons) particles. Rate of decay a physical constant. It does not change in different enironments. Measured in 1/2 lives

At Death all there
5730 yrs 1/2 left
11,460yrs 1/4 left
17,000 yrs 1/8 left
Too low to Detect, about 40,000

6. K-Ar Dating
* Used to date volcanic events. Important to Quaternary studies, because can calibrate other methods (paleomag, in situ, varnish) and because may be stratigraphically related to key deposits.

* Potassium (K) common in minerals. 39K and 41K are stable. 40K is in small amounts (0.012%) and decays to 40Ca or 40Ar with a 1/2 life of 1.3 billion years. Ca more common than Ar, so Ar used.

* Age is 40K vs 40Ar. Assume when rock is molten, argon is driven out. So volcanic rocks contain no argon. (Can have excess argon problem). With time Ar-40 produced and retained.

* Younger limit is about 100,000 for basalts and 10,000 for rocks rich in potassium. Older limit is over a billion.

7. Uranium-Series
Encompasses the range of radiometric techniques based on the declay of Uranium-238 and Uranium-235 by emission of alpha particles.

Ideal Sample:
Chemically precipitated from a low temperature solution and not redissolved. Typically precipitated as calcium carbonate with Uranium in Solution.

Assumptions:
(1) At the time of formation of a dated sample, the parent isotope(s) was present, but the daughter in question was either absent or present at a known activity level
(2) After a long time, the activity of the daughter becomes equal to the parent...reaches radiocactive equilibrium
(3) Sample has not been chemically disturbed since it was formed.

Materials Dated:


Corals (Marine Terrace Chronologies)
Speleothems (low concentration of U, 300 ka limit)
Stopping & Starting reflect glaciatioNS
Travertine -- if dense, free of detritus
Tufa
Lacustrine Limestone
Calcrete (tested against K-Ar, not systematic, but...)
Mollusk Shells (old shoreline ages)
Can date magma, but much harder & rarely done for BC K-Ar

9. Paleomagnetism
The earth's magnetic field varies. The history of fluctuations are recorded by magnetic particles in rocks and sediments when they are deposited.

By dating (e.g. K-Ar, fission track) these deposits, can assign dates to these fluctuations. Therefore, can use these paleomagnetic fluctuations are correlation tools to date deposits elsewhere.

10. Obsidian (and tephra) Hydration Dating
* Obsidian glass will react with water and hydrate. The rind is seen in thin sections by a change in the refraction index in a microscope. The thickness of the rind increases with time and temp.

* Hydration starts when a fresh surface is exposured, by glacial abrasion? By new obsidian flow? By artifact manufacturing

* Hydration is NOT LINEAR; more log.

* Depends on temp, moisture, physical structure of glass,chemistry of glass

* Needs to be calibrated in each local area for each microsite

* Best use in archaeological dating and glacial events in volcanic areas. Obsidian pebbles in moraines in Yellowstone provide dating of glacial deposits to 140 ka (Bull Lake) and 25 ka (Pinedale), using Lava flows 114 ka, 179 ka to calibrate obsidian hydration

11. Thermoluminescence (TL)
* TL is the light emitted from a mineral crystal when it is heated

* TL is derived from exposure to ionizing radiation. Free electrons are produced by the decay of radioisotopes in the matrix.

* Free electrons are trapped in the crytal defects. The longer the crystal is exposed to radiation, the higher the trapped content, and the more TL when the sample is heated.

* Ideally, amount of light is a funcation of the length of time the sample has seen since it was last heated to the point where it would zero the TL.

USE:
*Pottery in archaeology
*sediments baked by lava
*calcite precipitation
* marine and terrestrial sediments, if the TL is "zero'd" by exposure to sunlight during weathering, detachment, and erosion.

12. Amino Acid Racemization (AAR)
* Chemical Dating Method, dependent on time and temperature

* Amino acids are among the basic structures required by living organisms. Have amino groups (NH2) and carboxylic acid (COOH).

* Some amino acids are stable. Occur in similar amounts in recent and tertiary sheels of the same species.

* Others undergo RACEMIZATION, which is the transformation of a substance (with an asymmetric structure) to its mirror side, like racemic acid to tartaric acid)

* Rate of racemization is controlled by temp and time. If can guess at temperature, can estimate time. or establish correlative chronology

* need about 10 mg and measure in gas or liquid chromatography. Different AA labs typically complete inter-lab comparisons.

* The ratio of D/L in modern environments are pretty much zero, but increases with increasing age of fossils.

* AAR used in:


marine terrace studies
terrestrial river deposits
terrestrial loess deposits
paleosol organic mater

13. Soils as a Dating Tool Birkeland - Soil Stratigraphy

Field Properties: Depth of Solum, horizonation, color, texture consistency, structure, pH, clay films, carbonate

Lab Properties: particle size distribution, % OM loss on ignition, pH, dry color

PROBLEMS: Local Environment Erosion of soil horizons Aeolian input

Harden- Soil Index

BASIC APPROACH: one or more properties of a series of soils of differing ages are keyed to relative age values to produce a chronosequence. Then non-dated soils are assigned ages by comparison with the reference sequence

HARDEN Combines Soil Field (& can use lab) properties:


- soil thickness
-clay films
-texture plus wet consistence
- rubification (color hue & chroma)
- structure
- dry consistency
- moist consistency
- color value
- pH
- others, depending on type of soil structed

Assign points to each of these properties (like clay films, abundance, thickness, locaiton from 0-10-20-30-40.

Then normalize the point value for each property on scale 0-10

Found soil development has a semi-log relationship. Soil index from 0 to 1 (max) arithmatic and age log.

Ca-carbonate: Model, C-14, U-trend, U-series

14. Rock Varnish


- coatings on rock surfaces- AMS date organics
-systematic change in chemistry over time
- internal stratigraphy based on different microbal env.

15. In Situ Cosmogenic Isotopes

* Over 30 elements have radioisotopes with half-lives in the range of 1 ka to 100 myr. Many are within the range of interest to the Quaternary, 103 to 106.

* Five have been measured with AMS (Accelerator Mass Spectrometry) at natural levels. The idea is to use milligram samples of isotopes: C-14, 10-Be, Al-26, Cl-36, I-129

BASIC IDEA OF AMS: Each atomic species has a unique mass

-formation of a charge ion
- accelerate through electrostatic potential of MeVs (conventional mass spect uses KeVs)
- separate of ions based on mass-to-charge ratio
- measurement of number of ions in detectors

EXAMPLES OF USE:
AMS C-14:


* reduce sample size by 1000 milligrams to 1
* date individual seeds, pollen, ice core samples, individual tree rings, precious art objects
* trace carbon particulates in atms air pollution
* trace carbon cycle in ocean, biosphere, atmosphere
* with 1% precision, improve chronology of events
* In situ work in White Mtns, Antarctica, Hawaii

CHLORINE-36 (Fred Phillips)
* idea isotope for geomorphic studies BC 300,000 yr half-live In situ build-up can provide dating:


meteorite craters
glacial moraines
old shorelines
fault scarps
archaeological structures

* hydrology studies -- used for trace movements in Great Artesian Basin in Australia, high level nuclear waste siting, geothermal systems, bomb trace in infiltration studies

* continental saline sediments, Searles Lake, provide new reconstruction of climatic history

Al-26 * Use quarts from natural surfaces, because low AL concentration allows measurement of Al-25 buildup after about 1000 years.
* glacial polish in Sierra Nevada

Be-10 (in soils)
* depth profiles of Be-10 in ferromanganese nodules yield growth rates of 1-4 mm/million years. Also old ages for nodules
* can help determine long-term erosion history of landscapes

EXAMPLE OF USE: Merced River Terraces (Pavich, Harden) Be-10 retained in clays in top few meters. Decays there. Good technique until about 100 to 200 ka.

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